Magnetic field losses in Nd-Fe-B magnets under 10 MeV electron irradiation

Reversible changes in magnetic properties of Nd-Fe-B magnets under electron beam with the energy of 10 MeV and bremsstrahlung irradiation were investigated. It was shown that direct electron beam irradiation resulted in the decrease of magnetic flux and substantial alteration in the magnetic pattern...

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Datum:2017
Hauptverfasser: Bovda, V.A., Bovda, A.M., Guk, I.S., Dovbnya, A.N., Lyashchenko, V.N., Mytsykov, A.O., Onischenko, L.V., Kalinichenko, A.I., Kandybei, S.S., Repikhov, O.A.
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Veröffentlicht: Національний науковий центр «Харківський фізико-технічний інститут» НАН України 2017
Schriftenreihe:Вопросы атомной науки и техники
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Zitieren:Magnetic field losses in Nd-Fe-B magnets under 10 MeV electron irradiation / V.A. Bovda, A.M. Bovda, I.S. Guk, A.N. Dovbnya, V.N. Lyashchenko, A.O. Mytsykov, L.V. Onischenko, A.I. Kalinichenko, S.S. Kandybei, O.A. Repikhov // Вопросы атомной науки и техники. — 2017. — № 3. — С. 90-94. — Бібліогр.: 9 назв. — англ.

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spelling irk-123456789-1360952018-06-16T03:05:16Z Magnetic field losses in Nd-Fe-B magnets under 10 MeV electron irradiation Bovda, V.A. Bovda, A.M. Guk, I.S. Dovbnya, A.N. Lyashchenko, V.N. Mytsykov, A.O. Onischenko, L.V. Kalinichenko, A.I. Kandybei, S.S. Repikhov, O.A. Вычислительные и модельные системы Reversible changes in magnetic properties of Nd-Fe-B magnets under electron beam with the energy of 10 MeV and bremsstrahlung irradiation were investigated. It was shown that direct electron beam irradiation resulted in the decrease of magnetic flux and substantial alteration in the magnetic pattern on the surface of the samples. Increasing the radiation dose in 10 times did not lead to a linear reduction of magnetic flux. Bremsstrahlung also did not produce any significant drop in magnetic performance. Re-magnetization after the irradiation allowed to restore the initial magnetic properties of Nd-Fe-B magnets. Експериментально досліджений розподіл магнітного поля зразків магнітів, виготовлених з Nd-Fe-B сплаву, при опроміненні їх електронним пучком з енергією 10 МеВ, а також гальмівним випромінюванням такого пучка. Проведені дослідження показали, що величина і розподіл поля навколо магнітів змінюються при прямому опроміненні поверхні електронним пучком. Збільшення дози опромінення в 10 разів не приводить до лінійного зменшення поля зразка, який досліджувався. Під впливом гальмівного випромінювання електронів у зразку, розташованому поза впливом електронного пучка, істотної зміни магнітного поля не спостерігається. Повторне намагнічування зразка після опромінення електронним пучком дозволяє відновити первісну величину і розподіл поля навколо зразка. Экспериментально исследовано изменение магнитного поля образцов магнитов, изготовленных из Nd-Fe-B сплава, при облучении их электронным пучком с энергией 10 МэВ, а также тормозным излучением такого пучка. Проведенные исследования показали, что величина и распределение поля вокруг магнитов изменяются при прямом облучении поверхности электронным пучком. Увеличение дозы облучения в 10 раз не приводит к линейному изменению наблюдаемого изменения поля образца. Под воздействием тормозного излучения электронов в образце, расположенном вне воздействия электронного пучка, существенного изменения поля не наблюдается. Повторное намагничивание образца после облучения электронным пучком позволяет восстановить первоначальную величину и распределение поля вокруг образца. 2017 Article Magnetic field losses in Nd-Fe-B magnets under 10 MeV electron irradiation / V.A. Bovda, A.M. Bovda, I.S. Guk, A.N. Dovbnya, V.N. Lyashchenko, A.O. Mytsykov, L.V. Onischenko, A.I. Kalinichenko, S.S. Kandybei, O.A. Repikhov // Вопросы атомной науки и техники. — 2017. — № 3. — С. 90-94. — Бібліогр.: 9 назв. — англ. 1562-6016 PACS: 75.50.-y, 61.80.-x, 71.20.Eh http://dspace.nbuv.gov.ua/handle/123456789/136095 en Вопросы атомной науки и техники Національний науковий центр «Харківський фізико-технічний інститут» НАН України
institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
collection DSpace DC
language English
topic Вычислительные и модельные системы
Вычислительные и модельные системы
spellingShingle Вычислительные и модельные системы
Вычислительные и модельные системы
Bovda, V.A.
Bovda, A.M.
Guk, I.S.
Dovbnya, A.N.
Lyashchenko, V.N.
Mytsykov, A.O.
Onischenko, L.V.
Kalinichenko, A.I.
Kandybei, S.S.
Repikhov, O.A.
Magnetic field losses in Nd-Fe-B magnets under 10 MeV electron irradiation
Вопросы атомной науки и техники
description Reversible changes in magnetic properties of Nd-Fe-B magnets under electron beam with the energy of 10 MeV and bremsstrahlung irradiation were investigated. It was shown that direct electron beam irradiation resulted in the decrease of magnetic flux and substantial alteration in the magnetic pattern on the surface of the samples. Increasing the radiation dose in 10 times did not lead to a linear reduction of magnetic flux. Bremsstrahlung also did not produce any significant drop in magnetic performance. Re-magnetization after the irradiation allowed to restore the initial magnetic properties of Nd-Fe-B magnets.
format Article
author Bovda, V.A.
Bovda, A.M.
Guk, I.S.
Dovbnya, A.N.
Lyashchenko, V.N.
Mytsykov, A.O.
Onischenko, L.V.
Kalinichenko, A.I.
Kandybei, S.S.
Repikhov, O.A.
author_facet Bovda, V.A.
Bovda, A.M.
Guk, I.S.
Dovbnya, A.N.
Lyashchenko, V.N.
Mytsykov, A.O.
Onischenko, L.V.
Kalinichenko, A.I.
Kandybei, S.S.
Repikhov, O.A.
author_sort Bovda, V.A.
title Magnetic field losses in Nd-Fe-B magnets under 10 MeV electron irradiation
title_short Magnetic field losses in Nd-Fe-B magnets under 10 MeV electron irradiation
title_full Magnetic field losses in Nd-Fe-B magnets under 10 MeV electron irradiation
title_fullStr Magnetic field losses in Nd-Fe-B magnets under 10 MeV electron irradiation
title_full_unstemmed Magnetic field losses in Nd-Fe-B magnets under 10 MeV electron irradiation
title_sort magnetic field losses in nd-fe-b magnets under 10 mev electron irradiation
publisher Національний науковий центр «Харківський фізико-технічний інститут» НАН України
publishDate 2017
topic_facet Вычислительные и модельные системы
url http://dspace.nbuv.gov.ua/handle/123456789/136095
citation_txt Magnetic field losses in Nd-Fe-B magnets under 10 MeV electron irradiation / V.A. Bovda, A.M. Bovda, I.S. Guk, A.N. Dovbnya, V.N. Lyashchenko, A.O. Mytsykov, L.V. Onischenko, A.I. Kalinichenko, S.S. Kandybei, O.A. Repikhov // Вопросы атомной науки и техники. — 2017. — № 3. — С. 90-94. — Бібліогр.: 9 назв. — англ.
series Вопросы атомной науки и техники
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fulltext MAGNETIC FIELD LOSSES IN Nd− Fe−B MAGNETS UNDER 10MeV ELECTRON IRRADIATION V.A.Bovda, A.M.Bovda, I. S.Guk∗, A.N.Dovbnya, V.N.Lyashchenko, A.O.Mytsykov, L.V.Onischenko, A. I.Kalinichenko, S. S.Kandybei, O.A.Repikhov National Science Center ”Kharkiv Institute of Physics and Technology”, 61108, Kharkiv, Ukraine (Received April 10, 2017) Reversible changes in magnetic properties of Nd−Fe−B magnets under electron beam with the energy of 10MeV and bremsstrahlung irradiation were investigated. It was shown that direct electron beam irradiation resulted in the decrease of magnetic flux and substantial alteration in the magnetic pattern on the surface of the samples. Increasing the radiation dose in 10 times did not lead to a linear reduction of magnetic flux. Bremsstrahlung also did not produce any significant drop in magnetic performance. Re-magnetization after the irradiation allowed to restore the initial magnetic properties of Nd− Fe−B magnets. PACS: 75.50.-y, 61.80.-x, 71.20.Eh 1. INTRODUCTION Rare-earth permanent magnets are widely used in the self-powered compact devices [1,2]. Now, Nd−Fe−B magnets are the essential part of technological elec- tron accelerators with energy up to 10MeV . Mag- nets have many practical applications as focusing beam systems and energy beam measuring devices [3,4]. However, the stability of magnetic performance can be influenced by the direct electron beam and bremsstrahlung irradiation [5]. In this paper, we present the study of magnetic performance stabil- ity of Nd − Fe − B magnets under electron and bremsstrahlung irradiation. Nd − Fe − B mag- nets were manufactured using PLP technology [6,7]. KUT-1 technological accelerator [8] with the energy of 10MeV was used as the source of the electron beam. The density of magnetic samples obtained with PLP technology was 7.35...7.4 g/cm3. The mag- nets had geometrical dimensions of 30×40×12mm3. The surface of the samples was covered with a thin layer of nickel to prevent corrosion. During the ir- radiation, the samples were cooled with water at a temperature of no more than 40◦C. Pulsed magnetic field of 3.5T was used for samples magnetization. 2. EXPERIMENTAL SETUP The direct irradiation experiments were carried out with three magnets designates as M1, M4 and M5. All samples were located behind output foil of the accelerator. Continued water cooling was used to pre- vent samples from heating. The side (30×40mm2) of South magnetic pole (S. pole) was chosen for the di- rect electron irradiation. The heterogeneity of beam density was less than 10%. The M2 sample under- went bremsstrahlung radiation generated by electron bombardment of M1 sample. In view of this, M2 sample was placed beyond electron beam. The dis- tance between M1 and M2 samples was 1 cm. The M2 sample was also water-cooled. The non-irradiated M3 sample was used for reference measurements of induced activity and magnetic flux stability. M1, M2 and M4 samples were exposed to continue irradia- tion within 20hours. The absorbed dose of M1 and S4 samples was 16Grad. M5 sample was irradiated within 20hours sessions with 24 hours breaks. The total absorbed dose for M5 sample was 160Grad. The γ-spectra of each irradiated sample were col- lected within 24hours after the end of irradiation. CANBERRA GC1818 spectrometer with high-purity Ge semiconductor detector was utilized. As a result of 148Nd(γ, n)147Nd reaction with the threshold of 7.3MeV , the unstable 174Nd isotope with 10.98 days half-life was revealed. The 174Nd isotope attributes to 91.136, 319.406, 439.835, 530.913 keV . However, 174Nd isotope did not considerably change the activ- ity of the samples in comparison with non-irradiated one. Thus, negligible induced activity enables to use Nd − Fe − B magnets at the technological electron accelerators. 3. MAGNETIC MEASUREMENTS Magnetic measurements were performed by the seven (7) Hall probes assembly [9]. Hall probes were fixed in the copper matrix to temperature compensation. The distance between Hall probes was 6mm. The normal component of the magnetization was mea- sured. The relative accuracy was not less than 0.01%. ∗Corresponding author E-mail address: guk@kipt.kharkov.ua 90 ISSN 1562-6016. PROBLEMS OF ATOMIC SCIENCE AND TECHNOLOGY, 2016, N3(109). Series: Nuclear Physics Investigations (68), p.90-94. Magnetic samples were moved parallel to the surface of the copper matrix. The distance between mag- nets and copper matrix was 3.05mm. The steps of measurements along the direction of travel varied from 3 to 5mm. The accuracy of travel was 1µm. Initial reference point was fixed by the supporting system. The magnetic field distribution (magnetic flux) was scanned from the both sides of the magnet (30× 40mm2). Fig.1 shows the North pole (N. pole) magnetic scans for M1 sample before irradiation. Fig.1. Magnetic field scans for M1 sample (N. pole) Scanned data were used for the three-dimension square interpolation. The area of simulation was limited by the out-to-out Hall probes positions in the copper matrix and scanning area. Fig.2 demon- strates the simulation for the M1 sample utilizing data shown in Fig.1. Fig.2. Simulation of magnetic flux for M1 sample (N. pole) The magnetic field around the sample can be de- scribed by the integral Bx component in a plane 3.05mm of the surface of the block. The in- tegral Bx component of magnetic flux measured at the N. pole side of non-irradiated samples is shown in Table. It was revealed, that inte- gral Bx component of magnetic fluxes at both sides of the non-irradiated samples showed good agreement within the accuracy of measurements. Integral value of magnetic flux of the samples Name Integral Bx component Name (N. pole) , arb. units M1 175.763 M2 179.556 M3 175.452 M4 174.275 M5 176.357 The carried out examinations accuracy of recurring of integral Bx component for the same sample, re- lated to a binding to boundaries of the sample of a measuring system, give repeatability at level of 0.5%. 4. RESULTS AFTER ELECTRON IRRADIATION The simulation of magnetic field distribution for the sample after electron irradiation is shown in Figs.3-8. The simulation of the magnetic field distribution of M1 for S. pole is depicted in Fig.4. The corresponding integral Bx component of M1 sample for S. pole was −160.2. It can be seen that integral Bx component for M1 equals to 162.356 for N. pole. As it can be seen in Figs.3 and 4, the magnetic field distribution of both N. and S. poles are in a good agreement after electron irradiation, within the accuracy of measure- ments. Simulated magnetic field distribution for M4 sam- ple (N. pole) after irradiation is shown in Fig.5. It was revealed that integral Bx component (N. pole) for M4 sample after irradiation dropped to 151.122. The shape of the simulated magnetic field distribu- tion of S. pole for M4 sample is close to the pattern in the Fig.5. The integral Bx component of S. pole for M4 sample is about −151.509. Fig.3. The simulation of magnetic field distribution for M1 sample (N. pole) after irradiation (accumu- lated dose 16Grad) 91 Fig.4. Simulated magnetic field distribution for M1 sample (S. pole) after irradiation Fig.5. The simulation of magnetic field distribution for M4 sample (N. pole) after irradiation (accumu- lated dose 16Grad) Whereas direct electron irradiation substantially modified the magnetic pattern of the samples, bremsstrahlung irradiation hardly changed the magnetic field distribution (see Fig.6) and inte- gral Bx component of 178.526 (see also Table). Fig.6. Simulated magnetic field distribution N. pole of M2 sample Predictably, the most transformation of mag- netic field distribution was found for M5 sample with the highest accumulated dose of 160Grad (Fig.7). The integral Bx component was reduced to 126.556. It should be noted that integral Bx compo- nent was not proportional to the accumulated dose. Fig.7. Magnetic field distribution for M5 sam- ple (N. pole) after irradiation (accumulated dose 160Grad) 5. EFFECTS OF ACTION OF AN EXTERIOR MAGNETIC FIELD The full recovery of magnetic properties was indi- cated for M1 and M4 samples after re-magnetization. Figs.8-10 shows the simulated magnetic field distribu- tion of M1 and M5 samples after re-magnetization. After irradiation (see Fig.3) and re-magnetization (Fig.8) of M1 sample, the pattern of N. pole mag- netic field distribution was slightly changed and al- most coincided with the initial state (see Fig.1). The integral Bx component was about 175.224, which is in good agreement with the initial value. Fig.8. Magnetic field distribution N. pole of M1 sample after irradiation and re-magnetization. The same effect was indicated for M5 sample (see Figs.9 and 10). The integral Bx component of M5 sample after re-magnetization recovered to the initial value of 174.894 (N. pole) and −176.78 (S. pole). 92 Fig.9. Magnetic field distribution N. pole of M5 sample after irradiation and re-magnetization Fig.10. Magnetic field distribution S. pole of M5 sample after irradiation and re-magnetization 6. SUMMARY The direct electron irradiation of the Nd-Fe-B mag- nets let to the substantial change in magnetic field distribution of the samples. There was no direct correlation between the decrease of magnetic prop- erties and the accumulated dose within the range of 16...160Grad. Re-magnetization of the samples after irradiation resulted in the full recovery of magnetic properties. Within the interval of the used radiation absorption doses of the electron beam, no dependence of this effect on the dose was observed. Within the indicated doses, there was no significant change in the activity of the samples due to the formation of unstable isotopes in the material of magnets, which makes it possible to simplify the use of finished prod- ucts on technological accelerators with energy of up to 10MeV . References 1. David J.McLaughlin, KennethR. Hogstrom, Robert L. Carver, JohnP.Gibbons, PoladM. Shikhaliev, KennethL. Matthews II, Taylor Clarke, Alexander Henderson, and Edison P. Liang. Permanent-magnet energy spectrom- eter for electron beams from radio-therapy accelerators // Medical Physics. 2015, v.42, N9, p.5517-5529. 2. A.M.Bovda I.S.Guk. A.N.Dovbnya, S.G.Kononenko, V.N. Lyashchenko, A.O.Mytsykov. Dipole magnet with a con- stant field for the accelerator ”EPOS” // Problems of Atomic Science and Technology. Ser. ”Nuclear Physics Investigations”. 2015, N6(100), p.13-17. 3. F. Bodker, L.O.Baandrup et al. Permanent mag- nets in accelerators can save energy, space and cost // Proceedings of IPAC2013, Shanghai, China, p.3511-3513. 4. I.S.Guk, A.O.Mytsykov. Select of parametres of an analyzing magnet for the technological accel- erator of electrons // XIV conference on a high- energy physics, nuclear physics and accelerators. Abstracts broshure, Kharkov, 2016, p.117. 5. A.N.Dovbnya, A.E.Tolstoy, A.M.Bovda, O.M.Utva, V.L.Uvarov, M.A.Krasnogolovets. Study on radiation resistance of permanent Nd − Fe − B-base magnets under continuous radiation conditions // Problems of Atomic Science and Technology. Series ”Nuclear Physics Investigations”. 1999, N3(34), p.48-49. 6. Yasuhiro Une and Masato Sagawa // J. Japan Inst. Metals. 2012, v.76, N1, p.12-16. 7. M. Sagawa // Proc. 21st Int. Workshop on Rare Earth Permanent Magnets and Their Applica- tions, Bled, Slovenia, 2010 / Ed. by S.Kobe and P.J.McGuiness, (Ljubljana: Jozef Stefan Insti- tute, 2010), p.183. 8. M.I. Ayzatsky, V.N.Boriskin, et al. THE NSC KIPT electron linacs - R and D. // Problems of Atomic Science and Technology. Series ”Nuclear Physics Investigations” (33). 2003, N2, p.19-25. 9. I.S.Guk, A.N.Dovbnya, S.G.Kononenko, V.N. Lyashchenko, A.Yu.Mytsykov, V.P.Romas’ko, A.S. Tarasenko, V.N. Shcherbinin. Dipole magnet of the en- ergy filter for the accelerator ”EPOS” // Problems of Atomic Science and Technology. Series ”Nuclear Physics Investigations” (79), 2012, N3, p.67-69. 93 ÈÑÑËÅÄÎÂÀÍÈÅ ÂËÈßÍÈß ÎÁËÓ×ÅÍÈß ÎÁÐÀÇÖΠNd− Fe−B ÌÀÃÍÈÒΠÝËÅÊÒÐÎÍÍÛÌ ÏÓ×ÊÎÌ Ñ ÝÍÅÐÃÈÅÉ 10 Ìý ÍÀ ÂÅËÈ×ÈÍÓ ÏÎËß ÂÎÊÐÓà ÌÀÃÍÈÒÀ Â.À.Áîâäà, À.Ì.Áîâäà, È.Ñ.Ãóê, À.Í.Äîâáíÿ, Â.Í.Ëÿùåíêî, À.Î.Ìûöûêîâ, Ë.Â.Îíèùåíêî, À.È.Êàëèíè÷åíêî, Ñ.Ñ.Êàíäûáåé, Î.À.Ðåïèõîâ Ýêñïåðèìåíòàëüíî èññëåäîâàíî èçìåíåíèå ìàãíèòíîãî ïîëÿ îáðàçöîâ ìàãíèòîâ, èçãîòîâëåííûõ èç Nd− Fe−B ñïëàâà, ïðè îáëó÷åíèè èõ ýëåêòðîííûì ïó÷êîì ñ ýíåðãèåé 10 ÌýÂ, à òàêæå òîðìîçíûì èçëó÷åíèåì òàêîãî ïó÷êà. Ïðîâåäåííûå èññëåäîâàíèÿ ïîêàçàëè, ÷òî âåëè÷èíà è ðàñïðåäåëåíèå ïîëÿ âîêðóã ìàãíèòîâ èçìåíÿþòñÿ ïðè ïðÿìîì îáëó÷åíèè ïîâåðõíîñòè ýëåêòðîííûì ïó÷êîì. Óâåëè÷åíèå äîçû îáëó÷åíèÿ â 10 ðàç íå ïðèâîäèò ê ëèíåéíîìó èçìåíåíèþ íàáëþäàåìîãî èçìåíåíèÿ ïîëÿ îáðàçöà. Ïîä âîçäåéñòâèåì òîðìîçíîãî èçëó÷åíèÿ ýëåêòðîíîâ â îáðàçöå, ðàñïîëîæåííîì âíå âîçäåéñòâèÿ ýëåê- òðîííîãî ïó÷êà, ñóùåñòâåííîãî èçìåíåíèÿ ïîëÿ íå íàáëþäàåòñÿ. Ïîâòîðíîå íàìàãíè÷èâàíèå îáðàçöà ïîñëå îáëó÷åíèÿ ýëåêòðîííûì ïó÷êîì ïîçâîëÿåò âîññòàíîâèòü ïåðâîíà÷àëüíóþ âåëè÷èíó è ðàñïðåäå- ëåíèå ïîëÿ âîêðóã îáðàçöà. ÄÎÑËIÄÆÅÍÍß ÂÏËÈÂÓ ÎÏÐÎÌIÍÅÍÍß ÇÐÀÇÊI Nd− Fe−B ÌÀÃÍIÒI ÅËÅÊÒÐÎÍÍÈÌ ÏÓ×ÊÎÌ Ç ÅÍÅÐÃI�Þ 10 Ìå ÍÀ ÂÅËÈ×ÈÍÓ ÏÎËß ÍÀÂÊÎËÎ ÌÀÃÍIÒÓ Â.Î.Áîâäà, Î.Ì.Áîâäà, I.Ñ.Ãóê, À.Ì.Äîâáíÿ, Â.Ì.Ëÿùåíêî, À.Î.Ìèöèêîâ, Ë.Â.Îíiùåíêî, Î. I.Êàëiíi÷åíêî, Ñ.Ñ.Êàíäèáåé, Î.Î.Ðåïiõîâ Åêñïåðèìåíòàëüíî äîñëiäæåíèé ðîçïîäië ìàãíiòíîãî ïîëÿ çðàçêiâ ìàãíiòiâ, âèãîòîâëåíèõ ç Nd−Fe−B ñïëàâó, ïðè îïðîìiíåííi ¨õ åëåêòðîííèì ïó÷êîì ç åíåðãi¹þ 10 ÌåÂ, à òàêîæ ãàëüìiâíèì âèïðîìiíþ- âàííÿì òàêîãî ïó÷êà. Ïðîâåäåíi äîñëiäæåííÿ ïîêàçàëè, ùî âåëè÷èíà i ðîçïîäië ïîëÿ íàâêîëî ìàãíiòiâ çìiíþþòüñÿ ïðè ïðÿìîìó îïðîìiíåííi ïîâåðõíi åëåêòðîííèì ïó÷êîì. Çáiëüøåííÿ äîçè îïðîìiíåííÿ â 10 ðàçiâ íå ïðèâîäèòü äî ëiíiéíîãî çìåíøåííÿ ïîëÿ çðàçêà, ÿêèé äîñëiäæóâàâñÿ. Ïiä âïëèâîì ãàëüìiâ- íîãî âèïðîìiíþâàííÿ åëåêòðîíiâ ó çðàçêó, ðîçòàøîâàíîìó ïîçà âïëèâîì åëåêòðîííîãî ïó÷êà, iñòîòíî¨ çìiíè ìàãíiòíîãî ïîëÿ íå ñïîñòåðiãà¹òüñÿ. Ïîâòîðíå íàìàãíi÷óâàííÿ çðàçêà ïiñëÿ îïðîìiíåííÿ åëåê- òðîííèì ïó÷êîì äîçâîëÿ¹ âiäíîâèòè ïåðâiñíó âåëè÷èíó i ðîçïîäië ïîëÿ íàâêîëî çðàçêà. 94