Dose distribution in the heterogeneous materials irradiated by electron beams

The simulation of the absorbed depth-dose distribution (DDD) near the boundary of contacting materials with a different density and/or by effective atomic numbers of materials irradiated by a scanning electron beam was fulfilled. The experimental validation of the obtained theoretical predictions...

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Datum:2004
Hauptverfasser: Kaluska, I., Lazurik, V.T., Lazurik, V.M., Popov, G.F., Rogov, Y.V., Zimek, Z.
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Sprache:English
Veröffentlicht: Національний науковий центр «Харківський фізико-технічний інститут» НАН України 2004
Schriftenreihe:Вопросы атомной науки и техники
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Zitieren:Dose distribution in the heterogeneous materials irradiated by electron beams / I. Kaluskab, V.T. Lazurika, V.M. Lazurika, G.F. Popova, Y.V. Rogova, Z. Zimek // Вопросы атомной науки и техники. — 2004. — № 1. — С. 184-186. — Бібліогр.: 3 назв. — англ.

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spelling irk-123456789-790682015-03-26T03:01:55Z Dose distribution in the heterogeneous materials irradiated by electron beams Kaluska, I. Lazurik, V.T. Lazurik, V.M. Popov, G.F. Rogov, Y.V. Zimek, Z. Применение ускоренных пучков The simulation of the absorbed depth-dose distribution (DDD) near the boundary of contacting materials with a different density and/or by effective atomic numbers of materials irradiated by a scanning electron beam was fulfilled. The experimental validation of the obtained theoretical predictions related with abnormal behavior of the DDD in heterogeneous materials was fulfilled on the radiation-technological lines with Linac LAE 13/9, INCT. Проведено моделювання розподілу поглиненої дози (РПД) на границі контактуючих матеріалів з різними щільностями і/чи атомними номерами, що опромінюються скануючим електронним пучком. Експериментальну перевірку теоретичних передбачень аномальної поведінки РПД у гетерогенних матеріалах проводили на радіаційно-технологічній лінії з лінійним прискорювачем електронів LAE 13/9, ІЯХТ, Варшава, Польща. Проведено моделирование распределения поглощенной дозы (РПД) на границе раздела веществ с различными плотностями и/или атомными номерами, облучаемых сканирующим электронным пучком. Экспериментальную проверку теоретических предсказаний аномального поведения РПД в гетерогенных материалах проводили на радиационно-технологической линии с линейным ускорителем электронов LAE 13/9, ИЯХТ, Варшава, Польша. 2004 Article Dose distribution in the heterogeneous materials irradiated by electron beams / I. Kaluskab, V.T. Lazurika, V.M. Lazurika, G.F. Popova, Y.V. Rogova, Z. Zimek // Вопросы атомной науки и техники. — 2004. — № 1. — С. 184-186. — Бібліогр.: 3 назв. — англ. 1562-6016 PACS: 81.70.-q http://dspace.nbuv.gov.ua/handle/123456789/79068 en Вопросы атомной науки и техники Національний науковий центр «Харківський фізико-технічний інститут» НАН України
institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
collection DSpace DC
language English
topic Применение ускоренных пучков
Применение ускоренных пучков
spellingShingle Применение ускоренных пучков
Применение ускоренных пучков
Kaluska, I.
Lazurik, V.T.
Lazurik, V.M.
Popov, G.F.
Rogov, Y.V.
Zimek, Z.
Dose distribution in the heterogeneous materials irradiated by electron beams
Вопросы атомной науки и техники
description The simulation of the absorbed depth-dose distribution (DDD) near the boundary of contacting materials with a different density and/or by effective atomic numbers of materials irradiated by a scanning electron beam was fulfilled. The experimental validation of the obtained theoretical predictions related with abnormal behavior of the DDD in heterogeneous materials was fulfilled on the radiation-technological lines with Linac LAE 13/9, INCT.
format Article
author Kaluska, I.
Lazurik, V.T.
Lazurik, V.M.
Popov, G.F.
Rogov, Y.V.
Zimek, Z.
author_facet Kaluska, I.
Lazurik, V.T.
Lazurik, V.M.
Popov, G.F.
Rogov, Y.V.
Zimek, Z.
author_sort Kaluska, I.
title Dose distribution in the heterogeneous materials irradiated by electron beams
title_short Dose distribution in the heterogeneous materials irradiated by electron beams
title_full Dose distribution in the heterogeneous materials irradiated by electron beams
title_fullStr Dose distribution in the heterogeneous materials irradiated by electron beams
title_full_unstemmed Dose distribution in the heterogeneous materials irradiated by electron beams
title_sort dose distribution in the heterogeneous materials irradiated by electron beams
publisher Національний науковий центр «Харківський фізико-технічний інститут» НАН України
publishDate 2004
topic_facet Применение ускоренных пучков
url http://dspace.nbuv.gov.ua/handle/123456789/79068
citation_txt Dose distribution in the heterogeneous materials irradiated by electron beams / I. Kaluskab, V.T. Lazurika, V.M. Lazurika, G.F. Popova, Y.V. Rogova, Z. Zimek // Вопросы атомной науки и техники. — 2004. — № 1. — С. 184-186. — Бібліогр.: 3 назв. — англ.
series Вопросы атомной науки и техники
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fulltext DOSE DISTRIBUTION IN THE HETEROGENEOUS MATERIALS IRRADIATED BY ELECTRON BEAMS I. Kaluskab, V.T. Lazurika, V.M. Lazurika, G.F. Popova, Y.V. Rogova, Z. Zimekb aKharkov National University, Kharkov, Ukraine; bInstitute of Nuclear Chemistry and Technology, INCT, Warsaw, Poland; E-mail: popov@univer.kharkov.ua The simulation of the absorbed depth-dose distribution (DDD) near the boundary of contacting materials with a different density and/or by effective atomic numbers of materials irradiated by a scanning electron beam was fulfilled. The experimental validation of the obtained theoretical predictions related with abnormal behavior of the DDD in heterogeneous materials was fulfilled on the radiation-technological lines with Linac LAE 13/9, INCT. PACS: 81.70.-q 1. INTRODUCTION The numerical investigations of a dose distribution in heterogeneous targets irradiated on radiation-techno- logical lines (RTL) by a scanned electron beams on moving conveyer were carried out with use of software ModeRTL [1]. The software ModeRTL (Modeling of the Radiation-Technological Line) is developed for sim- ulation of radiation processes and calculation of the ab- sorbed dose, temperature, and charge distribution within products irradiated by a scanning electron beam with the electron energy range from 0.1 to 20 MeV on industrial RTL. Investigations were fulfilled in the two-dimensional geometrical model, in which the target on a conveyor line was represented as a set of parallelepipeds unlimit- ed on length along a motion of the conveyor (axis Z). It is supposed, that the parallelepiped sides are oriented only in parallel and perpendicularly to scanning direc- tion of an electron beam (axis Y), and the material of each element of target (represented as separate paral- lelepiped) is homogeneous. Dose fields in a plane of scanning of an electron beam (plane XY) were calculat- ed. Depth-dose distributions (depth is measured from an irradiated surface of object along an axis X perpendicu- lar to axis Y) were compared on various distances from a boundary of materials with different densities and/or atomic numbers. The comparison and analysis of the results have al- lowed one to bring out a series of features in behavior of dependence of a depth-dose distribution near to bound- ary of two different materials. Let us note, that an anomaly dose which appear near the boundaries of two materials with different atomic numbers are well known. As a rule, the consideration of these effects is perform for a case of normal falling of an electron beam and at a uniform irradiation of a boundary of contacting materials, i.e. in one-dimensional model. In this case, the influence of density of the contacting materials on value of boundary effects can be neglected. This report is focused mainly to boundary effects of another sort, namely, boundary effects appearing due to difference of densities of contacting materials. 2. THEORETICAL PREDICTIONS The heterogeneous target consisting of two blocks was chosen for an illustration of some theoretical pre- dictions, obtained on the basis of results analysis of computer experiments. Blocks of contacting materials have identical chemical composition and different densi- ties. For example, such target can be easily implemented with use of homogeneous (PE density of 0.94 g/cm3) and granules (PE2 bulk density of 0.3 g/cm3) polyethylene. The geometrical parameters of a target were chosen so that the curves of depth-dose distribution at center of blocks corresponded to an extreme case of a semi-infinite target. It is implemented when the sizes of blocks greater than r0 – continuous slowing-down approximation range of electrons in material of the block. The key features of simulation results of an electron dose distribution in targets consisting of two materials with different density are the following: 1. Depth-dose distribution near to boundaries of the contacting materials with different density differs under the shape from a depth-dose distribution in semi-infinite target for each of contacting materials. 2. The values of doses near to boundary of two ma- terials which differed only in density coincide on a sur- face of a target and can differ in depth of a target, 3. The value of a dose in material with smaller den- sity is greater than in material with greater density on all depth of an irradiated target, 4. Maximal values of a dose near to a boundary of the contacting materials with different density can ex- ceed maximal values of a dose in semi-infinite target for each of contacting materials, 5. The local minimum in depth-dose distribution can appear on small distances from a surface of a target in material with greater density, 6. Depth-dose distribution near to boundaries of con- tacting materials with different density have the similar shapes on considerable distances from a surface of a tar- get. The theoretical analysis of mentioned above general features allows to make a conclusion about a determina- tive role of electrons, which move along boundary, in process of formation of a boundary effect. It is important for development of theoretical models to utilize an experimental validation of basic features of boundary effects predicted on the basis of computer simulation of an irradiation process. The quality of an irradiation process in radiation technologies are deter- mined by values of the dose limits - Dmin and Dmax. The practical recommendations and conclusions obtained on the basis of the mentioned above basic features of boundary effects are important for radiation technolo- gies. Thus, the theoretical predictions require experi- ___________________________________________________________ PROBLEMS OF ATOMIC SIENCE AND TECHNOLOGY. 2004. № 1. Series: Nuclear Physics Investigations (42), p.184-186. 184 mental validation on actual RTL. 3. EXPERIMENTAL The experimental investigations of the absorbed depth-dose distribution near to boundary of two materi- als with different density and/or by effective atomic number which were irradiated by a scanning electron beam with energy 10 МеV were fulfilled. The absorbed dose for irradiated materials was delivered in the range of 40…60 kGy. The experiments were performed on the RTL with Linac LAE 13/9 at the INCT, Warsaw, Poland [2]. Dose effects near to boundary of two con- tacting materials with different density and atomic num- ber such as Al with density 2,7 g/cm3, high density polyethylene (PE) block with density 0.94 g/cm3, PE1 granules with bulk density 0.66 g/cm3, and wood with density 0,44 g/cm3 were investigated. The materials were represented as parallelepipeds at which the con- tacting boundaries are in parallel with an axis of elec- trons beam. Cellulose Triacetate (CTA) dosimetric film (FTR-125) with thickness 0.125 mm, density 1.32 g/cm3 was used for measurement of a depth-dose distribution. 4. RESULTS AND DISCUSSION Results of the specially carried out dose distribution measurements in CTA films inserted in the standard Al dosimetric wedge (the points) and obtained with use of the software ModeRTL (histograms) are presented in Fig.1,a. Results of Monte Carlo simulation of the depth- dose distributions in homogeneous materials (his- tograms with points +) and obtained by semi-empirical model [3] for semi-infinite medium (dash line) are pre- sented for comparison in Fig. 1,a,b. As it is seen from Fig. 1,a, the ratio of calculated values of a dose in CTA film to a dose in Al on a sur- face of a target (x=0, see values in the first cells of two histograms) corresponds to the ratio of values of a dose measured by Al dosimetric wedge (Experiment 1) to calculated values of a dose in Al (histogram with points +) on any depth in a target. Difference of a dose profile in a CTA film from a dose profile in target material are determined by two factors: by change of a dose profile due to differences of stopping powers of materials (first factor) and change of a dose profile due to differences of materials density (second factor). The smaller density and greater stopping power of CTA film material relatively Al corresponds to a case, when both factors work in one direction, that lead to considerable excess of a dose distribution in CTA films relatively a dose in Al (greater than 20%). The differ- ence in density of a film material and the target materi- als lead to appreciable distortion of a dose profile in a film (compare curves of a dose - measured by Al dosi- metric wedge (Experiment 1) and calculated (or mea- sured) in CTA films). It essentially distinguishes a case, when there is a difference in densities of contacting materials from a case, when there is a difference only in stopping powers of material. The conclusions formulated on the basis of the visu- al analysis presented on Fig.1,a are agreed with experi- mental and simulation results for PE granules (See Fig. 1,b). The ratio of a stopping power of CTA film material to a stopping power of PE is less than 1 and density of CTA film material more than PE density. Fig.1. Depth-dose distribution in the target consisting of two Al blocks (a) and PE1 blocks (PE1 density 0.66 g/cm3) (b): Histograms - results of calculations by a method Monte Carlo of the dose distribution in Al and PE1 blocks (points +) and in CTA film placed between two Al and PE1 blocks; Dashed line - dose distribution calculated with the use semi-empirical model at the cen- ter of Al and PE1 blocks. Experimental results for dose distribution measured by CTA film placed between two Al and PE1 blocks are shown by points Differences of a dose profile in a CTA film from a dose profile in bulk PE are determined by two factors, as well as for a case of CTA film in Al. However, in this case, action of the factors is opposite and the values of difference of doses in CTA film and in bulk PE less on an absolute value and has an opposite sign. Results of Monte Carlo simulation (histograms) of the depth-dose distributions on the boundary of two contacting blocks consisting of different materials and obtained by semi-empirical model for semi-infinite medium (solid line) are presented in Fig. 2,a and b. Experimental results for depth-dose distribution measured by CTA film placed between materials with different density in Fig. 2,a and b are shown by points. The relative accuracy of experimental data did not ex- ceed 5% for values of doses greater than 10 kGy. The uncertainty of the depth value of all curves is 0.125 cm and the average size in each point is 0.1см. It is sup- posed, that the process of an irradiation can be described in one-dimensional model, i.e. the effects of lateral boundaries of a target can be neglected. ___________________________________________________________ PROBLEMS OF ATOMIC SIENCE AND TECHNOLOGY. 2004. № 1. Series: Nuclear Physics Investigations (42), p.184-186.185 The requirements for experiments and computer modeling were chosen so that in dedicated range of depths the level of precision for an experimental and calculation data (relative deviation) of measuring no greater than 5%, relative root-mean-square statistical er- ror no greater than 5%) was supplied sufficient for car- rying out of the comparative analysis. Fig.2. Depth-dose distribution in the target consists of PE-Al (a) (PE density 0.94 g/cm3) and wood-PE blocks (b) (wood density 0.44 g/cm3): Histograms – results of calculations by a method Monte Carlo of the depth-dose distribution near to boundary of Al, PE, and wooden blocks; Solid curves – depth-dose distribution at the center of Al, PE, and wooden and PE blocks calculated with the use semi-empirical model. Xopt is the optimum target thickness for PE and wooden blocks at one-sided irradiation respectively As it is seen in Fig.2,a and b in dedicated range of target depths the measurement results are satisfactorily agreed with results obtained on the basis of simulation of an irradiation process by a Monte-Carlo method. It is possible to conclude, that basic features of boundary effects which were described in items 1,3,4,6 (part «Introduction») obtained theoretically with using the software ModeRTL are experimentally validated. The established fact of strong distortion of a dose pro- file in thin dosimetric film (see Fig.1,a and b) specifies necessity of modernization of a measurement principles for experimental validation of items 2,4 for the list of general features of boundary effects. The results represented in Fig.2,a and b concerned to a case when the sizes of the contacting materials in a di- rection perpendicular to a boundary of target are great and it is possible to suppose a target by unlimited. 5. CONCLUSIONS The experimental and theoretical examinations of boundary anomalies of a dose distribution are per- formed on model samples. Both used materials (Al, PE, wood, CTA film) and radiation facility on basis of the LAE 13/9 are typical for a series of radiation technolo- 186 gies. As it is seen from comparison of experimental re- sults with data, obtained by simulation methods, fol- lows, that the theoretical predictions of behavior of a dose near to a boundary of two materials with different density are correct. It was established, that the boundary anomalies of a dose can be realized at radiation process- ing of heterogeneous materials. Investigation of those anomalies can be used to estimate the quality of an irra- diation fulfilled on RTL. It is shown that an application of designed software model for planning of irradiation on RTL and interpreta- tion of results obtained by dosimetric film is correct, is useful and, in a series of cases it is necessary in practice. REFERENCES 1. V.T. Lazurik, V.M. Lazurik, G. Popov, Yu. Rogov. Proc. of EBT’03 Conf. Varna, Bulgaria, p.616-622. 2. Z. Zimek, S. Kołyga, V.M. Levin, V.M. Nikolaev, V.V. Rumyantsev, L.P. Fomin. An Institute of Nuc- lear Research Electron Linac. // Nukleonika, 1972, v. 17, № 1-2, р. 67-75. 3. V.M. Lazurik, T. Tabata, V.T. Lazurik // Radiat. Phys. Chem. 2001, v. 60, р. 161-162. РАСПРЕДЕЛЕНИЕ ДОЗЫ В ГЕТЕРОГЕННЫХ МАТЕРИАЛАХ, ОБЛУЧАЕМЫХ ПУЧКАМИ ЭЛЕКТРОНОВ И. Калуска, В.Т. Лазурик, В.М. Лазурик, Г.Ф. Попов, Ю.В. Рогов, З. Зимек Проведено моделирование распределения поглощенной дозы (РПД) на границе раздела веществ с раз- личными плотностями и/или атомными номерами, облучаемых сканирующим электронным пучком. Экспе- риментальную проверку теоретических предсказаний аномального поведения РПД в гетерогенных материа- лах проводили на радиационно-технологической линии с линейным ускорителем электронов LAE 13/9, ИЯХТ, Варшава, Польша. РОЗПОДІЛ ДОЗИ В ГЕТЕРОГЕННИХ МАТЕРІАЛАХ, ЩО ОПРОМІНЮЮТЬСЯ ПУЧКАМИ ЕЛЕКТРОНІВ І. Калуска, В.Т. Лазурік, В.М. Лазурік, Г.Ф. Попов, Ю.В. Рогов, З. Зімек Проведено моделювання розподілу поглиненої дози (РПД) на границі контактуючих матеріалів з різними щільностями і/чи атомними номерами, що опромінюються скануючим електронним пучком. Експериментальну перевірку теоретичних передбачень аномальної поведінки РПД у гетерогенних матеріалах проводили на радіаційно-технологічній лінії з лінійним прискорювачем електронів LAE 13/9, ІЯХТ, Варшава, Польща. ___________________________________________________________ PROBLEMS OF ATOMIC SIENCE AND TECHNOLOGY. 2004. № 1. Series: Nuclear Physics Investigations (42), p.184-186.187 3. EXPERIMENTAL