Parametric instability influence on isotope separation by ion-cyclotron resonance method

Solution of the dispersion equation for linear potential ion cyclotron oscillations with characteristic parameters used for selective ion cyclotron resonance separation of gadolinium isotopes has revealed the presence of the shortwavelength unstable oscillation in the ion cyclotron frequency range...

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Дата:2006
Автори: Olshansky, V.V., Stepanov, K.N.
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Мова:English
Опубліковано: Національний науковий центр «Харківський фізико-технічний інститут» НАН України 2006
Назва видання:Вопросы атомной науки и техники
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Цитувати:Parametric instability influence on isotope separation by ion-cyclotron resonance method / V.V. Olshansky, K.N. Stepanov // Вопросы атомной науки и техники. — 2006. — № 6. — С. 204-206. — Бібліогр.: 4 назв. — англ.

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Digital Library of Periodicals of National Academy of Sciences of Ukraine
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spelling irk-123456789-823042015-05-28T03:02:16Z Parametric instability influence on isotope separation by ion-cyclotron resonance method Olshansky, V.V. Stepanov, K.N. Low temperature plasma and plasma technologies Solution of the dispersion equation for linear potential ion cyclotron oscillations with characteristic parameters used for selective ion cyclotron resonance separation of gadolinium isotopes has revealed the presence of the shortwavelength unstable oscillation in the ion cyclotron frequency range. Computer simulation of this instability by means of macro particle technique has shown that this instability may be responsible for turbulent heating of both resonant and nonresonant ions obtaining large transversal energy. It can decrease the efficiency of this method. 2006 Article Parametric instability influence on isotope separation by ion-cyclotron resonance method / V.V. Olshansky, K.N. Stepanov // Вопросы атомной науки и техники. — 2006. — № 6. — С. 204-206. — Бібліогр.: 4 назв. — англ. 1562-6016 PACS: 52.35.-g; 52.35.Mw; 28.60.+s http://dspace.nbuv.gov.ua/handle/123456789/82304 en Вопросы атомной науки и техники Національний науковий центр «Харківський фізико-технічний інститут» НАН України
institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
collection DSpace DC
language English
topic Low temperature plasma and plasma technologies
Low temperature plasma and plasma technologies
spellingShingle Low temperature plasma and plasma technologies
Low temperature plasma and plasma technologies
Olshansky, V.V.
Stepanov, K.N.
Parametric instability influence on isotope separation by ion-cyclotron resonance method
Вопросы атомной науки и техники
description Solution of the dispersion equation for linear potential ion cyclotron oscillations with characteristic parameters used for selective ion cyclotron resonance separation of gadolinium isotopes has revealed the presence of the shortwavelength unstable oscillation in the ion cyclotron frequency range. Computer simulation of this instability by means of macro particle technique has shown that this instability may be responsible for turbulent heating of both resonant and nonresonant ions obtaining large transversal energy. It can decrease the efficiency of this method.
format Article
author Olshansky, V.V.
Stepanov, K.N.
author_facet Olshansky, V.V.
Stepanov, K.N.
author_sort Olshansky, V.V.
title Parametric instability influence on isotope separation by ion-cyclotron resonance method
title_short Parametric instability influence on isotope separation by ion-cyclotron resonance method
title_full Parametric instability influence on isotope separation by ion-cyclotron resonance method
title_fullStr Parametric instability influence on isotope separation by ion-cyclotron resonance method
title_full_unstemmed Parametric instability influence on isotope separation by ion-cyclotron resonance method
title_sort parametric instability influence on isotope separation by ion-cyclotron resonance method
publisher Національний науковий центр «Харківський фізико-технічний інститут» НАН України
publishDate 2006
topic_facet Low temperature plasma and plasma technologies
url http://dspace.nbuv.gov.ua/handle/123456789/82304
citation_txt Parametric instability influence on isotope separation by ion-cyclotron resonance method / V.V. Olshansky, K.N. Stepanov // Вопросы атомной науки и техники. — 2006. — № 6. — С. 204-206. — Бібліогр.: 4 назв. — англ.
series Вопросы атомной науки и техники
work_keys_str_mv AT olshanskyvv parametricinstabilityinfluenceonisotopeseparationbyioncyclotronresonancemethod
AT stepanovkn parametricinstabilityinfluenceonisotopeseparationbyioncyclotronresonancemethod
first_indexed 2025-07-06T08:48:49Z
last_indexed 2025-07-06T08:48:49Z
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fulltext 204 Problems of Atomic Science and Technology. 2006, 6. Series: Plasma Physics (12), p. 204-206 PARAMETRIC INSTABILITY INFLUENCE ON ISOTOPE SEPARATION BY ION-CYCLOTRON RESONANCE METHOD V.V. Olshansky, K.N. Stepanov National Science Center “Kharkov Institute of Physics and Technology”, Akademicheskaya Str. 1, 61108, Kharkov, Ukraine Solution of the dispersion equation for linear potential ion cyclotron oscillations with characteristic parameters used for selective ion cyclotron resonance separation of gadolinium isotopes has revealed the presence of the short- wavelength unstable oscillation in the ion cyclotron frequency range. Computer simulation of this instability by means of macro particle technique has shown that this instability may be responsible for turbulent heating of both resonant and nonresonant ions obtaining large transversal energy. It can decrease the efficiency of this method. PACS: 52.35.-g; 52.35.Mw; 28.60.+s 1. INTRODUCTION According to this method [1] in the plasma coming with the thermal velocity from an ion source into the heating region under the antenna the resonant ions which are to be separated obtain their transverse energy from the RF field under the ion cyclotron resonance and are heated up on the average. The nonresonant ions obtain lesser energy due to Doppler effect and one can neglect their heating if the generator frequency (more precisely the magnetic field) is matched so that Tici VkVk 0||||0||0 >>⋅−− ωω , where ||V is the particle velocity along the magnetic field, TiV is its thermal velocity, Lk /20|| π= , L is the antenna length. Transverse RF field speeds up the resonant particles and they are heated. For a nonresonant particle the cyclotron frequency differs from one for a resonant particle by the value ( )AA∆=∆ 0ωω , where A is the atomic number of the isotope, and the condition of resonant absorption is not met for them, if ( )( )AAVLL Ti ∆=>> 08 ωπ . (1) In the RF field during the time TiVkt ||1~∆ the resonant ions obtain the current velocity of the order of ( )Tiires VkmeEu 0||02π≈ , where 0E is the complex amplitude of the field rotating in the direction of cyclotron gyration of ions. Current velocity of nonresonant ions will be of the order of ( ) ( )AABeEunores ∆⋅00 /~ . The velocity resu can be, by virtue of inequality (1), considerably greater than the velocity of nonresonant ions. If the relative velocity of resonant and nonresonant ions will become of the order of initial thermal velocity of ions, then in such plasma, due to the relative oscillations of ions, parametric instabilities will arise associated with potential ion cyclotron oscillations [2]. In the present work the linear growth rates of the parametric ion cyclotron instability, conditioned by the oscillations of different species ions, are found and computer simulation, based on the macro particle model (2D2V model [3]), of this instability is carried out for the gadolinium isotopes. 2. LINEAR THEORY OF PARAMETRIC ION CYCLOTRON INSTABILITIES Let us consider the particle motion in the pumping field [ ]( )tzki 00||0 (expRe ω−= EE that is switched on at the moment 0=t . Because the particle displacement is small in comparison with the antenna radius, then one can consider the electric field to be uniform. Integrating the equations of motion, neglecting small longitudinal electric field ||E and carrying out the averaging over initial Maxwell distribution, we obtain the expression for the average transversal velocity of particles ( ) ( ) ( )[ ]{ ( ) , 2 222 exp exp exp 2 0|| 0 0|| 0|| 0 2 0|| 0 0|| 0             − −         − − ⋅         −× ×−− − =⊥ α α α α αα α α α α ωω ωω ωω ωπ T c T T cT c T caa Vk W tVk i Vk W tVk ti Vk tiEme V (2) where yx iVVV ααα +=⊥ is the transversal velocity in the complex form, αωc is the ion cyclotron frequency of the ion of α -species, 0E is the complex amplitude of the pumping field, 0ω is the frequency of this field, that is equal to the cyclotron frequency of the ion species under separation. In expression (2) ( ) ( ) ( )         +⋅−= ∫ z dtti k k zzW 0 2 0|| 0||2 exp2 || exp π . In [4] the device was proposed for isotope gadolinium-157 separation with the parameters: 0B =3 T, 0n =1012 cm-3, initial temperature of ions is 10 eV, L =2 m, the frequency of alternating field is rescωω = =2⋅106 s-1, the plasma radius is 10 cm, the electric field strength is ϕE =3 V/cm. In this case resu ~3·106 cm/s, the nonresonant ions velocity is approximately 2 times smaller; the initial thermal velocity of ions is TiV ~2.5·105 cm/s. In Fig. 1 the dependence against time t0ωτ = of the velocities of the gadolinium isotopes G157 and G158 and their relative velocity, divided by the initial thermal velocity of ions, is shown for the conditions given above [4]. Oscillations of the relative velocity of the isotopes lead to the appearance of the amplitude beats with the pe- riod ( ) 3102 ≈∆=′ AAπτ , that arise from “instantaneous” switching on of the pumping field. At the initial stage the velocity growth is almost the same for the isotopes of different species. At the stage, when the relative velocity 205 of different isotopes is close to the maximum value, oscillations of the components of the transversal velocity take place in opposite phase. In this case the value of the relative velocity achieves 20 TiV . If switching on of the pumping field takes place at the moment −∞→t , then the oscillations with the frequency ciω disappear. Only the oscillations with the frequency 0ω remain. In this case the relative amplitude u at 400≥τ is equal to 4 TiV approximately. tc1ω 1/ TVu 11 / TVV 12 / TVV Fig. 1. Time dependence of the velocities of the gadoli- nium isotopes G157 ( 1V ), G158 ( 2V ) and their relative velocity u divided by the initial thermal velocity of Gd157 ( 1TV ) 0.5 1.0 1.5 kρ1 0.4 0.6 0.8 1.0 1.2 ω /ω c1 0.00 0.04 0.08 0.12 γ/ ω c1 γ/ωc1 ω/ωc1 Fig. 2. Dependence of frequencies and growth rates of the unstable oscillations against wave number ( 1|| ρk = 0.01). For oscillations with larger ||k growth rate is 1.5÷3 times less than maximal one The dispersion equation for unstable oscillations has a form of the infinite determinant that is equal to zero 0||det =mnA , (3) ( ) ( ) ( ) ( )0 0,1 1 ωωδε ωωδε δ α α p aJaJ m A p anpamp e mnmn +× × ++ += ∑ ∑ ∞ −∞= ++k , where αa is the displacement of ions of α -species in the pumping field, multiplied by the wave vector of the unstable oscillations, ( )αaJ p is the Bessel functions of the first kind, αδε is the contribution to the longitudinal plasma permittivity of the particles of α -species in the presence of the oscillations with the average velocity (2). The solution of the dispersion equation (3) for the parameters [4] in the case of the rest plasma, 0|| =V , is presented in Fig. 2 (it is assumed in computations, that nonresonant ions have a mass of the gadolinium-158 and concentration 0.843, and concentration of gadolinium-157 is equal to its concentration in the natural mixture, 0.157). In Fig. 2 there are two branches of the unstable oscillations, the frequencies of which join the ion cyclotron frequencies (because heavy ions are considered the difference of their cyclotron frequencies is negligible). One can see, that in the region 1≈ikρ ( iρ - is the Larmor radius of the ions) the difference between unstable oscillations frequencies and the frequency ciωω =0 is ciωω 05.0≈∆ . The growth rates have a maximum at 1~ikρ . The growth rate of the branch with lesser frequency achieves the value ciω06.0 , and the growth rate of the branch with larger frequency achieves the value ciω025.0 . The longitudinal wave number is small, ik ρ|| =0.01, but it exceeds the longitudinal wave number of the pumping field 0||k =0.03 cm-1 three times, that allows to neglect the pumping field nonuniformity . 3. COMPUTER SIMULATION RESULTS Two-dimensional numerical simulation of nonlinear evolution of the parametric ion cyclotron instability by macro particle technique was carried out for the ions of gadolinium isotopes with the parameters [4]. As distinct from the previous section we will assume, that the oscillations of the ions of different species are defined by formulae (2) with 00|| →k . In this case the velocity of the resonant isotopes, for which ωω =resc , will grow linearly with time, ( ) tBEcV ⋅= 001 / , and the simulation results obtained can be used up to the time lesser than ( ) 1 0|| −=∆ TiVkt , i.e. 300≈∆⋅ trescω . In Fig. 3 the time dependence of the averaged energy density of unstable oscillations of the electric field is shown with the initial value ( ) 3 00 100 −⋅= TnWE . 0 50 100 150 200 ωc1t 0.00 0.01 0.02 0.03 0.04 W E/ n 0 T Fig. 3. Time dependence of energy density of the self consistent electric field π82EWE = divided by the initial thermal energy density 206 The frequencies of these oscillations are of the order of cinω . The characteristic wave numbers at 20≤tciω are large, 1>ikρ . At the large time the oscillations are excited with 1~<ikρ . Note, the dependence of the value 00TnWE against time is nonlinear. It relates to the variation of the current velocities of the particles in time and nonlinear effects in the particles motion in the electric field of unstable oscillations. 0 50 100 150 200 ωp1t 0 1 2 3 4 5 6 7 8 T/ T 1 0 Fig. 4. Time dependence of the averaged chaotic energy of ions of the isotope Gd157 divided by its initial value Development of the parametric instability is accompanied by heating the particles. It is illustrated by Fig. 4. In Fig. 4 the time dependence of the relation of transversal chaotic energy of the resonant isotope G157 to the initial temperature is shown. At 180=tciω this value exceeds the initial value seven times. The heating is conditioned by nonlinearity of the equations of the particles motion and by the dynamic chaos that can arise. In Fig. 4 at 50>tciω one can see the oscillations with the frequency ciω2 and with the amplitude growing in time. It is related to high energy ions generation. Transversal chaotic energy of the nonresonant isotope G158 grows in time too and it has the value of the order of that is obtained for the G157isotope. 4. CONCLUSIONS On the ground of computer simulation by means of macro particle technique it is shown, that for the typical parameter values of plasma, magnetic field and alternating electric filed under condition of the ion cyclotron resonance for the gadolinium isotopes mixture, the small-scale potential ion cyclotron oscillations with transversal wave number of the order of the inverse Larmor radius of ions arise in plasma as a result of the parametric instability after the relative velocity of the different isotopes achieves the value of the order of their thermal velocity. This instability results in the turbulent heating of both resonant and nonresonant ions and it can reduce the efficiency of the isotope separation method given. REFERENCES 1. Yu.A. Muromkin. Razdeleniye izotopov v plazme s pomoschyu ionno-tsiklotonnogo nagreva // Itogi nauki i tekhniki. Series: “Fizika Plazmy”. M: VINITI, 1991, N 12, p. 83. 2. K. N. Stepanov. Non-Linear Parametric Phenomena during Radio Frequency Heating in the Ion Cyclotron Frequency Range // Plasma Physics and Controlled Fusion. 1996, v. 38, N 12, p. A13. 3. V.V. Ol’shansky. KC-A Kinetic Computer Code for Investigation of Parametric Plasma Instabilities // Seibersdorf Report, Juli 1995, OEFZS-4752, Seibersdorf, Austria. 4. V. I. Volosov, I. A. Kotel’nikov, S. G. Kuz’min. O razdelenii izotopov tyazhelyh elementov metodom izotopicheski selektivnogo ICR-nagreva // Fizika Plazmy. 1998, v. 24, N 6, p. 517. . , . , , . , , , , . . , . , , . , , , , .